The pressure dependence of the Curie temperature T-C(P) in La0.75Ca0.25MnO3 was determined by neutron diffraction up to 8 GPa, and compared with the metallization temperature T-IM(P) (Postorino et al 2003 Phys. Rev. Lett. 91 175501). The behavior of the two temperatures appears similar over the whole pressure range, suggesting a key role of magnetic double-exchange also in the pressure regime where the superexchange interaction is dominant. The coexistence of antiferromagnetic and ferromagnetic peaks at high pressure and low temperature indicates a phase separated regime which is well reproduced with a dynamical mean-field calculation for a simplified model. A new P-T phase diagram has been proposed on the basis of the whole set of experimental data. RI Capone, Massimo/A-7762-2008

Pressure induced magnetic phase separation in La0.75Ca0.25MnO3 manganite

Capone, Massimo;
2012-01-01

Abstract

The pressure dependence of the Curie temperature T-C(P) in La0.75Ca0.25MnO3 was determined by neutron diffraction up to 8 GPa, and compared with the metallization temperature T-IM(P) (Postorino et al 2003 Phys. Rev. Lett. 91 175501). The behavior of the two temperatures appears similar over the whole pressure range, suggesting a key role of magnetic double-exchange also in the pressure regime where the superexchange interaction is dominant. The coexistence of antiferromagnetic and ferromagnetic peaks at high pressure and low temperature indicates a phase separated regime which is well reproduced with a dynamical mean-field calculation for a simplified model. A new P-T phase diagram has been proposed on the basis of the whole set of experimental data. RI Capone, Massimo/A-7762-2008
2012
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4
1
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045601
https://arxiv.org/abs/1112.1927
Baldini, M; Capogna, L; Capone, Massimo; Arcangeletti, E; Petrillo, C; Goncharenko, I; Postorino, P.
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/20.500.11767/12226
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