In the atomic force microscope, the nanoscale force topography of even complex surface superstructures is extracted by the changing vibration frequency of a scanning tip. An alternative dissipation topography with similar or even better contrast has been demonstrated recently by mapping the (x,y) -dependent tip damping but the detailed damping mechanism is still unknown. Here we identify two different tip dissipation mechanisms: local mechanical softness and hysteresis. Motivated by recent data, we describe both of them in a one-dimensional model of Moiré superstructures of incommensurate overlayers. Local softness at "soliton" defects yields a dissipation contrast that can be much larger than the corresponding density or corrugation contrast. At realistically low vibration frequencies, however, a much stronger and more effective dissipation is caused by the tip-induced nonlinear jumping of the soliton, naturally developing bistability and hysteresis. Signatures of this mechanism are proposed for experimental identification
AFM dissipation topography of soliton superstructures in adsorbed overlayers / Negri, C; Manini, N; Vanossi, A; Santoro, Giuseppe Ernesto; Tosatti, Erio. - In: PHYSICAL REVIEW. B, CONDENSED MATTER AND MATERIALS PHYSICS. - ISSN 1098-0121. - 81:4(2010), pp. 045417.1-045417.5. [10.1103/PhysRevB.81.045417]
AFM dissipation topography of soliton superstructures in adsorbed overlayers
Santoro, Giuseppe Ernesto;Tosatti, Erio
2010-01-01
Abstract
In the atomic force microscope, the nanoscale force topography of even complex surface superstructures is extracted by the changing vibration frequency of a scanning tip. An alternative dissipation topography with similar or even better contrast has been demonstrated recently by mapping the (x,y) -dependent tip damping but the detailed damping mechanism is still unknown. Here we identify two different tip dissipation mechanisms: local mechanical softness and hysteresis. Motivated by recent data, we describe both of them in a one-dimensional model of Moiré superstructures of incommensurate overlayers. Local softness at "soliton" defects yields a dissipation contrast that can be much larger than the corresponding density or corrugation contrast. At realistically low vibration frequencies, however, a much stronger and more effective dissipation is caused by the tip-induced nonlinear jumping of the soliton, naturally developing bistability and hysteresis. Signatures of this mechanism are proposed for experimental identificationFile | Dimensione | Formato | |
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